246 research outputs found
Photodissociation of the {HeH} molecular ion
The photodissociation cross section of the molecular ion HeH was
calculated within the Born-Oppenheimer approximation for a parallel, a
perpendicular, and an isotropic orientation of the molecular axis with respect
to the field, considering also different initial vibrational and rotational
states. The results were compared to recent data from a free-electron laser
experiment performed at the FLASH facility [H.B. Pedersen {\it et al.}, Phys.
Rev. Lett. 98, 223202, (2007)]. Within the experimental uncertainties
theoretical and experimental results are compatible with each other.Comment: 16 pages, 8 figure
Alignment-Dependent Ionization of Molecular Hydrogen in Intense Laser Fields
The alignment dependence of the ionization behavior of H exposed to
intense ultrashort laser pulses is investigated on the basis of solutions of
the full time-dependent Schr\"odinger equation within the fixed-nuclei and
dipole approximation. The total ionization yields as well as the
energy-resolved electron spectra have been calculated for a parallel and a
perpendicular orientation of the molecular axis with respect to the
polarization axis of linear polarized laser pulses. For most, but not all
considered laser peak intensities the parallel aligned molecules are easier to
ionize. Furthermore, it is shown that the velocity formulation of the
strong-field approximation predicts a simple interference pattern for the ratio
of the energy-resolved electron spectra obtained for the two orientations, but
this is not confirmed by the full ab initio results.Comment: 4 figure
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